This is the closest grocery-esque store to my place in Little Italy. The array of foods that they have here is amazing. I have never bought anything perishable here, except for a dessert (I had to laugh when the employee informed me that it wasn't 100% organic or warned me that it wasn't healthy!), so I can't comment about the produce or anything, but I've always been really pleased with the canned goods that I've purchased. The prices are sorta high, but that's to be expected given the nature of the goods they sell. Too bad, though, because I (and many people, probably) would love to eat more organically if we could afford it! Unfortunately, they do have some gaping holes in their product line, but I suspect that it's due to the fact they're an organic store.
One caveat: do not purchase the Erehwon Raisin Bran and expect it to taste like good ole' Kellogg's Raisin Bran. Well, it will if you add approximately three bags of sugar...