Every pastry I have tried here is good but the twice baked Chocolate, Almond and Pistachio croissants are the best to me. They also seem to sell out the fastest. If you want to make sure that you have your choice of the full selection of the pastries, it's better to go early in the morning. The evenings are the most crowded and they run out of a lot of items. They also offer breakfast sandwiches.
There is a smaller location Uptown that has a more limited pastry selection. They really need to build more of these in other parts of Charlotte too :-)