This is the only place I get coffee anymore. Hands-down my favourite cafe in the city.
The coffee (ask about the Armenian coffee - they make it perfectly, and import the beans from an Armenian supplier in San Francisco) is consistently amazing, with a variety of delicious snacks (2 cheese flatbread is killer) and deserts (baklava is some of the best you can find in downtown TO) to indulge in.
The ambiance is super friendly, with tasteful and mildly eccentric decor which helps set this place apart from some of the other cafes around it. The bathroom hosts one of the coolest mirrors in the city. Of course, other than the exceptionally good coffee, food, and design, the thing that makes this place stand out is the fact that they have a wicked vinyl collection to browse through as you wait for your order.
The owners and staff are a pleasure to chat with, and happy to answer any questions or offer recommendations. Can't recommend this place enough.